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山西省某地区土壤多环芳烃污染特征、来源解析及风险评价

Pollution Characteristics, Source Apportionment and Risk Assessment of Polycyclic Aromatic Hydrocarbons in Soil from A Certain Area of Shanxi Province

  • 摘要: 为准确了解山西省北部某地区土壤多环芳烃(PAHs)的污染特征、来源及其风险程度,对研究区土壤中的PAHs进行了污染特征分析,采用特征比值法对土壤PAHs进行了来源解析,并对土壤PAHs可能造成的生态及健康风险进行了评价。结果表明:研究区土壤中的16种PAHs总含量在2.74~782.34 ng/g之间;研究区土壤中PAHs的分布具有较强的空间变异性且高环PAHs变异性最强;研究区土壤中PAHs的主要来源为煤炭、生物质燃烧以及液体化石燃料燃烧,同时也存在部分石油源;研究区土壤中PAHs的污染呈现团块状、片状分布,污染严重区多为平原工矿企业集中地区;成人和儿童的健康风险受到的影响程度存在差异,两者皆存在潜在的致癌风险,但成人的致癌健康风险要高于儿童。

     

    Abstract: In order to accurately understand the pollution characteristics, sources and health risks of polycyclic aromatic hydrocarbons (PAHs) in the soil of a certain area in northern Shanxi Province, the pollution characteristics of PAHs in the soil of the study area were analyzed. The characteristic ratio method was used to analyze the sources of PAHs in the soil, and the possible health risks caused by PAHs in the soil were evaluated. The results showed that the total content of 16 PAHs in the soil of the study area was 2.74~782.34 ng/g. The distribution of PAHs in the soil of the study area had strong spatial variability, and the variability of high-ring PAHs was the strongest. The PAHs in the soil of the study area are mainly derived from coal, biomass combustion and liquid fossil fuel combustion, and there are also some oil sources. The soil PAHs pollution in the study area showed lumpy and flaky, and the serious pollution areas were mostly concentrated areas of industrial and mining enterprises in the plain. There are differences in the degree of impact on the health risks of adults and children. Both have potential carcinogenic risks, but the carcinogenic health risks of adults are higher than those of children.